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On the E-H transition in inductively coupled radio frequency oxygen plasmas: II. Electronegativity and the impact on particle kinetics
- Abstract In this series of two papers we present results about the E-H transition of an inductively coupled oxygen discharge driven at radio frequency (13.56 MHz) for different total gas pressures. The mode transition from the low density E-mode to the high density H-mode is studied using comprehensive plasma diagnostics. The measured electron density can be used to distinguish between the different operation modes. This paper focuses on the determination of the negative atomic ion density and the electronegativity by two experimental methods and global rate equation calculation. As a result, the electronegativity significantly decreases over two orders of magnitude from about 25 in the E-mode to about 0.1 in the H-mode. The temporal behavior of the electronegativity in pulsed ICP shows that the negative atomic ion density reaches a steady state after 10 ms. Negative atomic ions are mainly produced by the dissociative attachment with the molecular ground state. The ion–ion recombination with the positive molecular ions and the collisional detachment with the singlet molecular metastables contribute significantly to the loss of the negative atomic ions.
Author: | Thomas Wegner, Christian Küllig, Jürgen Meichsner |
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URN: | urn:nbn:de:gbv:9-opus-59195 |
DOI: | https://doi.org/10.1088/1361-6595/26/2/025007 |
ISSN: | 0963-0252 |
ISSN: | 1361-6595 |
Parent Title (English): | Plasma Sources Science and Technology |
Publisher: | IOP Publishing |
Document Type: | Article |
Language: | English |
Date of first Publication: | 2017/01/19 |
Release Date: | 2022/11/01 |
Tag: | electronegativity; inductively coupled plasma; laser photodetachment; microwave interferometry; mode transition; oxygen |
GND Keyword: | - |
Volume: | 26 |
Issue: | 2 |
Article Number: | 025007 |
Page Number: | 10 |
Faculties: | Mathematisch-Naturwissenschaftliche Fakultät / Institut für Physik |
Collections: | Artikel aus DFG-gefördertem Publikationsfonds |
Licence (German): | Creative Commons - Namensnennung |